Note: This answer is incomplete. An integral representation for the series is derived below, but it remains to be seen if that integral can be evaluated in turn.
Define the function $f:\mathbb{R}\rightarrow\mathbb{R}$ via the definite integral
$$\begin{align}
\mathcal{S}
&:=\sum_{n=1}^{\infty}\frac{H_{n-1}^{3}\left(-4\right)^{n}}{n^{2}\binom{2n}{n}}.\tag{1}\\
\end{align}$$
The $n$-th central binomial coefficient is defined through the factorial function for all nonnegative integers by
$$\binom{2n}{n}:=\frac{\left(2n\right)!}{\left(n!\right)^{2}};~~~\small{n\in\mathbb{Z}_{\ge0}}.$$
The reciprocals of the central binomial coefficients can be written in terms of the beta function. For each positive integer $n\in\mathbb{N}$, we have
$$\begin{align}
\frac{1}{\binom{2n}{n}}
&=\frac{\left(n!\right)^{2}}{\left(2n\right)!}\\
&=\frac{\left[\Gamma{\left(n+1\right)}\right]^{2}}{\Gamma{\left(2n+1\right)}}\\
&=\frac{\left[n\,\Gamma{\left(n\right)}\right]^{2}}{2n\,\Gamma{\left(2n\right)}}\\
&=\frac{n}{2}\cdot\frac{\left[\Gamma{\left(n\right)}\right]^{2}}{\Gamma{\left(2n\right)}}\\
&=\frac{n}{2}\mathrm{B}{\left(n,n\right)}.\\
\end{align}$$
Recall the definition of the beta function via the integral representation
$$\mathrm{B}{\left(a,b\right)}:=\int_{0}^{1}\mathrm{d}t\,t^{a-1}\left(1-t\right)^{b-1};~~~\small{a>0\land b>0}.$$
Using the technique of summing under the integral we can convert the infinite series $\mathcal{S}$ into a definite integral. We obtain
$$\begin{align}
\mathcal{S}
&=\sum_{n=1}^{\infty}\frac{H_{n-1}^{3}\left(-4\right)^{n}}{n^{2}\binom{2n}{n}}\\
&=-2\sum_{n=1}^{\infty}\frac{H_{n-1}^{3}\left(-4\right)^{n-1}}{n}\cdot\frac{2}{n\binom{2n}{n}}\\
&=-2\sum_{n=1}^{\infty}\frac{H_{n-1}^{3}\left(-4\right)^{n-1}}{n}\mathrm{B}{\left(n,n\right)}\\
&=-2\sum_{n=1}^{\infty}\frac{H_{n-1}^{3}\left(-4\right)^{n-1}}{n}\int_{0}^{1}\mathrm{d}t\,t^{n-1}\left(1-t\right)^{n-1}\\
&=-2\sum_{n=0}^{\infty}\frac{H_{n}^{3}\left(-4\right)^{n}}{n+1}\int_{0}^{1}\mathrm{d}t\,t^{n}\left(1-t\right)^{n}\\
&=-2\sum_{n=0}^{\infty}\frac{H_{n}^{3}\left(-1\right)^{n}}{n+1}\int_{0}^{1}\mathrm{d}t\,\left[4t\left(1-t\right)\right]^{n}\\
&=-4\sum_{n=0}^{\infty}\frac{H_{n}^{3}\left(-1\right)^{n}}{n+1}\int_{0}^{\frac12}\mathrm{d}t\,\left[4t\left(1-t\right)\right]^{n};~~~\small{symmetry}\\
&=-4\sum_{n=0}^{\infty}\frac{H_{n}^{3}\left(-1\right)^{n}}{n+1}\int_{0}^{1}\mathrm{d}x\,\frac{x^{n}}{4\sqrt{1-x}};~~~\small{\left[t=\frac{1-\sqrt{1-x}}{2}\right]}\\
&=-\sum_{n=0}^{\infty}\int_{0}^{1}\mathrm{d}x\,\frac{H_{n}^{3}\left(-x\right)^{n}}{\sqrt{1-x}}\cdot\frac{1}{n+1}\\
&=-\sum_{n=0}^{\infty}\int_{0}^{1}\mathrm{d}x\,\frac{H_{n}^{3}\left(-x\right)^{n}}{\sqrt{1-x}}\int_{0}^{1}\mathrm{d}y\,y^{n}\\
&=-\sum_{n=0}^{\infty}\int_{0}^{1}\mathrm{d}x\int_{0}^{1}\mathrm{d}y\,\frac{H_{n}^{3}\left(-xy\right)^{n}}{\sqrt{1-x}}\\
&=-\int_{0}^{1}\mathrm{d}x\int_{0}^{1}\mathrm{d}y\,\sum_{n=0}^{\infty}\frac{H_{n}^{3}\left(-xy\right)^{n}}{\sqrt{1-x}}\\
&=-\int_{0}^{1}\mathrm{d}x\,\frac{1}{\sqrt{1-x}}\int_{0}^{1}\mathrm{d}y\,\sum_{n=1}^{\infty}H_{n}^{3}\left(-xy\right)^{n}\\
&=-\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\int_{-x}^{0}\mathrm{d}t\,\sum_{n=1}^{\infty}H_{n}^{3}t^{n};~~~\small{\left[y=-x^{-1}t\right]}.\tag{2}\\
\end{align}$$
It can be demonstrated that
$$\begin{align}
\sum_{n=1}^{\infty}H_{n}^{3}z^{n}
&=-\frac{3S_{1,2}{\left(z\right)}-\operatorname{Li}_{3}{\left(z\right)}+3\ln{\left(1-z\right)}\operatorname{Li}_{2}{\left(z\right)}+\ln^{3}{\left(1-z\right)}}{\left(1-z\right)};~~~\small{z\in\left(-1,1\right)}.\tag{3}\\
\end{align}$$
Substituting this expression for the infinite series in the last line of $(3)$ above, and then using integration by parts to integrate the various terms of the inner-integral, we arrive at a single-variable definite integral representation for $\mathcal{S}$:
$$\begin{align}
\mathcal{S}
&=-\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\int_{-x}^{0}\mathrm{d}t\,\sum_{n=1}^{\infty}H_{n}^{3}t^{n}\\
&=\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\int_{-x}^{0}\mathrm{d}t\,\frac{3S_{1,2}{\left(t\right)}-\operatorname{Li}_{3}{\left(t\right)}+3\ln{\left(1-t\right)}\operatorname{Li}_{2}{\left(t\right)}+\ln^{3}{\left(1-t\right)}}{\left(1-t\right)}\\
&=\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\int_{-x}^{0}\mathrm{d}t\,\bigg{[}\frac{3S_{1,2}{\left(t\right)}}{1-t}-\frac{\operatorname{Li}_{3}{\left(t\right)}}{1-t}+\frac{3\ln{\left(1-t\right)}\operatorname{Li}_{2}{\left(t\right)}}{1-t}+\frac{\ln^{3}{\left(1-t\right)}}{1-t}\bigg{]}\\
&=\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\bigg{[}\int_{-x}^{0}\mathrm{d}t\,\frac{3S_{1,2}{\left(t\right)}}{1-t}-\int_{-x}^{0}\mathrm{d}t\,\frac{\operatorname{Li}_{3}{\left(t\right)}}{1-t}\\
&~~~~~+\int_{-x}^{0}\mathrm{d}t\,\frac{3\ln{\left(1-t\right)}\operatorname{Li}_{2}{\left(t\right)}}{1-t}+\int_{-x}^{0}\mathrm{d}t\,\frac{\ln^{3}{\left(1-t\right)}}{1-t}\bigg{]}\\
&=\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\bigg{[}-3\operatorname{Li}_{1}{\left(-x\right)}\,S_{1,2}{\left(-x\right)}+3\int_{-x}^{0}\mathrm{d}t\,\frac{\ln^{3}{\left(1-t\right)}}{2t}\\
&~~~~~+\operatorname{Li}_{1}{\left(-x\right)}\operatorname{Li}_{3}{\left(-x\right)}+\int_{-x}^{0}\mathrm{d}t\,\frac{\operatorname{Li}_{1}{\left(t\right)}\operatorname{Li}_{2}{\left(t\right)}}{t}\\
&~~~~~+\frac32\operatorname{Li}_{1}{\left(-x\right)}^{2}\operatorname{Li}_{2}{\left(-x\right)}-\frac32\int_{-x}^{0}\mathrm{d}t\,\frac{\ln^{3}{\left(1-t\right)}}{t}\\
&~~~~~+\frac14\ln^{4}{\left(1+x\right)}\bigg{]}\\
&=\int_{0}^{1}\mathrm{d}x\,\frac{1}{x\sqrt{1-x}}\bigg{[}3\ln{\left(1+x\right)}\,S_{1,2}{\left(-x\right)}-\ln{\left(1+x\right)}\operatorname{Li}_{3}{\left(-x\right)}\\
&~~~~~+\frac32\ln^{2}{\left(1+x\right)}\operatorname{Li}_{2}{\left(-x\right)}+\frac14\ln^{4}{\left(1+x\right)}-\frac12\operatorname{Li}_{2}{\left(-x\right)}^{2}\bigg{]}.\tag{4}\\
\end{align}$$