Let me point out that as others have observed we can spot the complexity right away without making much of an effort. It is clear that the contribution of the recursive term outgrows that of the work term. It is possible however to find an exact solution to a related recurrence that has the same complexity.
Suppose we have the following recurrence for $T(n)$ where $T(0)=0$, $T(1)=c_1$ and $T(2)=c_2$ and for $n\ge 3,$
$$T(n) = 4 T(\lfloor n/3 \rfloor) + n \lfloor\log \lfloor \log_3 n \rfloor\rfloor.$$
Furthermore suppose that the representation of $n$ in base three is given by
$$n = \sum_{k=0}^{\lfloor \log_3 n \rfloor} d_k 3^k.$$
Then it is not difficult to see that $T(n)$ for $n\ge 3$ has the exact closed form
$$T(n) = [d_{\lfloor \log_3 n \rfloor}=1] c_1 4^{\lfloor \log_3 n \rfloor}
+ [d_{\lfloor \log_3 n \rfloor}=2] c_2 4^{\lfloor \log_3 n \rfloor}
\\+ \sum_{j=0}^{\lfloor \log_3 n \rfloor-1}
\lfloor \log (\lfloor \log_3 n \rfloor - j) \rfloor
4^j \sum_{k=j}^{\lfloor \log_3 n \rfloor} d_k 3^{k-j}.$$
Now to get bounds on this we need an upper and a lower bound on the sum term. For an upper bound consider a string of two-digits, which gives
$$\sum_{j=0}^{\lfloor \log_3 n \rfloor-1}
\lfloor \log (\lfloor \log_3 n \rfloor - j) \rfloor
4^j \times 2 \times \sum_{k=j}^{\lfloor \log_3 n \rfloor} 3^{k-j}
\\ = \sum_{j=0}^{\lfloor \log_3 n \rfloor-1}
\lfloor \log (\lfloor \log_3 n \rfloor - j) \rfloor
4^j \times (3^{\lfloor \log_3 n \rfloor+1-j}-1)
\\ = \sum_{j=1}^{\lfloor \log_3 n \rfloor}
\lfloor \log j \rfloor
4^{\lfloor \log_3 n \rfloor-j} \times (3^{j+1}-1)
= 4^{\lfloor \log_3 n \rfloor}
\sum_{j=1}^{\lfloor \log_3 n \rfloor}
\lfloor \log j \rfloor
4^{-j} \times (3^{j+1}-1).$$
The sum term converges to a number, which is about $$6.271543822.$$
For a lower bound consider a one digit followed by a string of zeros, which gives
$$\sum_{j=0}^{\lfloor \log_3 n \rfloor-1}
\lfloor \log (\lfloor \log_3 n \rfloor - j) \rfloor
4^j \times 3^{\lfloor \log_3 n \rfloor -j}
\\ = \sum_{j=1}^{\lfloor \log_3 n \rfloor}
\lfloor \log j \rfloor
4^{\lfloor \log_3 n \rfloor-j} \times 3^j
= 4^{\lfloor \log_3 n \rfloor} \sum_{j=1}^{\lfloor \log_3 n \rfloor}
\lfloor \log j \rfloor (3/4)^j.$$
The sum term again converges to a number, which in this case is
$$2.097465834.$$
We are done with our investigation because both the upper and the lower bound term have been shown to consist entirely of contributions that are asymptotic to $4^{\lfloor \log_3 n \rfloor}$ (this includes the two terms in the leading digit Iverson bracket). Hence our final complexity is
$$ \Theta\left(4^{\lfloor \log_3 n \rfloor}\right)
= \Theta\left(4^{\log_3 n} \right)
= \Theta\left(3^{\log_3 4 \times \log_3 n}\right)
= \Theta\left(n^{\log_3 4}\right)$$
as predicted by inspection.
This MSE link features another Master Theorem computation that uses the same technique.