Let's correct your attempt. You made a systematic error, namely omitting cases with two disjoint pairs of adjacent $c$s. While most of your other terms are correct, there are some cases where you made computational errors. Since you did not explicitly state your cases, you will have to compare your terms with mine in order to identify those errors.
Also, I recommend including the $1$s in your multinomial coefficients both to avoid confusion with binomial coefficients and to make it easier to keep track of the number of objects.
A multinomial coefficient
$$\binom{n}{n_1, n_2, n_3, \cdots, n_k} = \frac{n!}{n_1! n_2 ! n_3! \cdots n_k!}$$
counts the number of distinguishable ways to arrange $n = n_1 + n_2 + n_3 + \cdots + n_k$ objects in a row if there are $n_1$ objects of type $1$, $n_2$ objects of type $2$, $n_3$ of type $3$, and so forth.
Since you appear to be using $S_i$ to denote arrangements with $i$ pairs of adjacent identical letters, I will denote the total number of arrangements by $S$ rather than $S_0$, since $S_0$, the number of arrangements with no pairs of adjacent identical letters, is what we want to find.
$S$: There are nine positions to fill, of which two are $a$s, three are $b$s, and four are $c$s. They can be filled in
$$|S| = \binom{9}{2}\binom{7}{3}\binom{4}{4} = \frac{9!}{2!3!4!} = \binom{9}{2, 3, 4}$$
ways since we must choose two of the nine positions for the $a$s, three of the remaining seven positions for the $b$s, and all four of the remaining four positions for the $c$s.
$S_1$: Your counts are all correct.
A pair of adjacent $a$s: We have eight objects to arrange: $aa, b, b, b, c, c, c, c$. They can be arranged in
$$\binom{8}{1, 3, 4}$$
ways.
A pair of adjacent $b$s: We have eight objects to arrange: $a, a, bb, b, c, c, c, c$. They can be arranged in
$$\binom{8}{2, 1, 1, 4}$$
ways.
A pair of adjacent $c$s: We have eight objects to arrange: $a, a, b, b, b, cc, c, c$. They can be arranged in
$$\binom{8}{2, 3, 1, 2}$$
ways.
Hence, $$|S_1| = \binom{8}{1, 3, 4} + \binom{8}{2, 1, 1, 4} + \binom{8}{2, 3, 1, 2}$$
$S_2$: You should have seven objects in all cases.
A pair of adjacent $a$s and a pair of adjacent $b$s: There are seven objects to arrange: $aa, bb, b, c, c, c, c$. They can be arranged in
$$\binom{7}{1, 1, 1, 4}$$
ways.
A pair of adjacent $a$s and a pair of adjacent $c$s: There are seven objects to arrange: $aa, b, b, b, cc, c, c$. They can be arranged in
$$\binom{7}{1, 3, 1, 2}$$
ways.
Two overlapping pairs of adjacent $b$s: There are seven objects to arrange: $a, a, bbb, c, c, c, c$. They can be arranged in
$$\binom{7}{2, 1, 4}$$
ways.
A pair of adjacent $b$s and a pair of adjacent $c$s: There are seven objects to arrange: $a, a, bb, b, cc, c, c$: They can be arranged in
$$\binom{7}{2, 1, 1, 1, 2}$$
ways.
Two overlapping pairs of adjacent $c$s: There are seven objects to arrange: $a, a, b, b, b, ccc, c$. They can be arranged in
$$\binom{7}{2, 3, 1, 1}$$
ways. Notice that $2 + 3 + 1 + 1 = 7$, which is a good way of checking whether you have the correct number of terms.
Two disjoint pairs of adjacent $c$s: There are seven objects to arrange: $a, a, b, b, b, cc, cc$. They can be arranged in
$$\binom{7}{2, 3, 2}$$
ways.
Hence, $$S_2 = \binom{7}{1, 1, 1, 4} + \binom{7}{1, 3, 1, 2} + \binom{7}{2, 1, 4} + \binom{7}{2, 1, 1, 1, 2} + \binom{7}{2, 3, 1, 1} + \binom{7}{2, 3, 2}$$
$S_3$: You should have six objects in all cases.
A pair of adjacent $a$s and two overlapping pairs of adjacent $b$s: We have six objects to arrange: $aa, bbb, c, c, c, c$. They can be arranged in
$$\binom{6}{1, 1, 4}$$
ways.
A pair of adjacent $a$s, a pair of adjacent $b$s, and a pair of adjacent $c$s: We have six objects to arrange: $aa, bb, b, cc, c, c$. They can be arranged in
$$\binom{6}{1, 1, 1, 1, 2}$$
ways.
A pair of adjacent $a$s and two overlapping pairs of adjacent $c$s: We have six objects to arrange: $aa, b, b, b, ccc, c$. They can be arranged in
$$\binom{6}{1, 3, 1, 1}$$
ways.
A pair of adjacent $a$s and two disjoint pairs of adjacent $c$s: We have six objects to arrange: $aa, b, b, b, cc, cc$. They can be arranged in
$$\binom{6}{1, 3, 2}$$
ways.
Two overlapping pairs of adjacent $b$s and a pair of adjacent $c$s: We have six objects to arrange: $a, a, bbb, cc, c, c$. They can be arranged in
$$\binom{6}{2, 1, 1, 2}$$
ways.
A pair of adjacent $b$s and two overlapping pairs of adjacent $c$s: We have six objects to arrange: $a, a, bb, b, ccc, c$. They can be arranged in
$$\binom{6}{2, 1, 1, 1, 1}$$
ways.
A pair of adjacent $b$s and two disjoint pairs of adjacent $c$s: We have six objects to arrange: $a, a, bb, b, cc, cc$. They can be arranged in
$$\binom{6}{2, 1, 1, 2}$$
ways.
Three overlapping pairs of adjacent $c$s: We have six objects to arrange: $a, a, b, b, b, cccc$. They can be arranged in
$$\binom{6}{2, 3, 1}$$
ways.
Hence,
$$|S_3| = \binom{6}{1, 1, 4} + \binom{6}{1, 1, 1, 1, 2}+ \binom{6}{1, 3, 1, 1} + \binom{6}{1, 3, 2} + \binom{6}{2, 1, 1, 2} + \binom{6}{2, 1, 1, 1, 1} + \binom{6}{2, 1, 1, 2} + \binom{6}{2, 3, 1}$$
$S_4$: You should have five objects in all cases.
A pair of adjacent $a$s, two overlapping pairs of adjacent $b$s, a pair of adjacent $c$s. We have five objects to arrange: $aa, bbb, cc, c, c$. They can be arranged in
$$\binom{5}{1, 1, 1, 2}$$
ways.
A pair of adjacent $a$s, a pair of adjacent $b$s, and two overlapping pairs of adjacent $c$s: We have five objects to arrange: $aa, bb, b, ccc, c$. Since the objects are distinct, they can be arranged in $5!$ ways.
A pair of adjacent $a$s, a pair of adjacent $b$s, and two disjoint pairs of adjacent $c$s: We have five objects to arrange: $aa, bb, b, cc, cc$. They can be arranged in
$$\binom{5}{1, 1, 1, 2}$$
ways.
A pair of adjacent $a$s and three overlapping pairs of adjacent $c$s: We have five objects to arrange: $aa, b, b, b, cccc$. They can be arranged in
$$\binom{5}{1, 3, 1}$$
ways.
Two overlapping pairs of adjacent $b$s and two overlapping pairs of adjacent $c$s: We have five objects to arrange: $a, a, bbb, ccc, c$. They can be arranged in
$$\binom{5}{2, 1, 1, 1}$$
ways.
Two overlapping pairs of adjacent $b$s and two disjoint pairs of adjacent $c$s: We have five objects to arrange: $a, a, bbb, cc, cc$. They can be arranged in
$$\binom{5}{2, 1, 2}$$
ways.
A pair of adjacent $b$s and three overlapping pairs of adjacent $c$s: We have five objects to arrange: $a, a, bb, b, cccc$. They can be arranged in
$$\binom{5}{2, 1, 1, 1}$$
ways.
Hence, $$|S_4| = \binom{5}{1, 1, 1, 2} + 5! + \binom{5}{1, 1, 1, 2} + \binom{5}{1, 3, 1} + \binom{5}{2, 1, 1, 1} + \binom{5}{2, 1, 2} + \binom{5}{2, 1, 1, 1}$$
$S_5$: You should have four objects in all cases.
A pair of adjacent $a$s, two overlapping pairs of adjacent $b$s, and two overlapping pairs of adjacent $c$s: We have four objects to arrange: $aa, bbb, ccc, c$. Since the objects are all distinct, they can be arranged in $4!$ ways.
A pair of adjacent $a$s, two overlapping pairs of adjacent $b$s, and two disjoint pairs of adjacent $c$s: We have four objects to arrange: $aa, bbb, cc, cc$. They can be arranged in
$$\binom{4}{1, 1, 2}$$
ways.
A pair of adjacent $a$s, a pair of adjacent $b$s, and three overlapping pairs of adjacent $c$s: We have four objects to arrange: $aa, bb, b, cccc$. Since the objects are all distinct, they can be arranged in $4!$ ways.
Two overlapping pairs of adjacent $b$s and three overlapping pairs of adjacent $c$s. We have four objects to arrange: $a, a, bbb, cccc$. They can be arranged in
$$\binom{4}{2, 1, 1}$$
ways.
Hence, $$|S_5| = 4! + \binom{4}{1, 1, 2} + 4! + \binom{4}{2, 1, 1}$$
$S_6$: You did this correctly.
A pair of adjacent $a$s, two overlapping pairs of adjacent $b$s, and two disjoint pairs of adjacent $c$s: We have three objects to arrange: $aa, bbb, cccc$. Since they are all distinct, they can be arranged in $$|S_6| = 3!$$ ways.
By the Inclusion-Exclusion Principle, the number of arrangements of $a, a, b, b, b, c, c, c, c$ in which no two adjacent letters are identical is
$$|S| - |S_1| + |S_2| - |S_3| + |S_4| - |S_5| + |S_6| = 79$$
in agreement with the answer true blue anil obtained by using the more advanced technique of the generalized Laguerre polynomial.