I've seen other answers to this question and wanted to take another approach to it. I'd appreciate some feedback:
Suppose said set was countable, then we can enumerate each bijection, say as $S:=\{f_n: \mathbb{N} \to \mathbb{N} | n\in \mathbb{N}\ \text{and } f_n \text{ is a bijection}\}$. Since each $f_n$ is bijective, can create the correspondence to its unique inverse: $$f_n \longleftrightarrow f_n ^{-1}$$
Consider the set of bijective inverses, $S':=\{f^{-1}_{n}: \mathbb{N} \to \mathbb{N} | n\in \mathbb{N}\ \text{and } f^{-1}_{n} \text{ is the inverse of} f_n \}$. Then it must be that $$S = S'$$,
otherwise, there is some inverse function $f_m^{-1}$ not in S, which would contradict the countability of $S$.
On the other hand, $S \subset S'$ means that for an arbitrary $n$, $f_n \in S'$, so there is some $m\in \mathbb{N}$ such that
$$f_n(x) = f_m ^{-1} (x) $$ for each x. This means that, $$f_m(f_n (x)) =x $$ So that $f_m$ is the inverse of $f_n$; but by construction of S', it must be that $m=n$. Since $n$ was arbitrary we have that each bijection is its own inverse, which means that for each $n$, $f_n=Id_{\mathbb{N}}$, the identity function on $\mathbb{N}$. Thus, $$S = \{Id_{\mathbb{N}}\}$$ a contradiction.