Using the well-known identity
$$\sum_{n=1}^\infty \frac{\binom{2n}n}{4^n}x^n=\frac{1}{\sqrt{1-x}}-1$$
Divide both sides by $x$ then integrate , we get
$$\quad\displaystyle\sum_{n=1}^\infty \frac{\binom{2n}n}{n4^n}x^n=-2\ln(1+\sqrt{1-x})+C $$
set $x=0,\ $ we get $C=2\ln2$
Then
$$\sum_{n=1}^\infty \frac{\binom{2n}n}{n4^n}x^n=-2\ln(1+\sqrt{1-x})+2\ln2\tag1$$
Multiply both sides of (1) by $-\frac{\ln(1-x)}{x}$ then integrate from $x=0$ to $1$ and use the fact that $-\int_0^1 x^{n-1}\ln(1-x)dx=\frac{H_n}{n}$ we get
\begin{align}
\sum_{n=1}^\infty\frac{H_n}{n^24^n}{2n\choose n}&=2\underbrace{\int_0^1\frac{\ln(1+\sqrt{1-x})\ln(1-x)}{x}dx}_{\sqrt{1-x}=y}-2\ln2\underbrace{\int_0^1\frac{\ln(1-x)}{x}dx}_{-\zeta(2)}\\
&=8\int_0^1\frac{y\ln(1+y)\ln y}{1-y^2}dy+2\ln2\zeta(2)\\
&=4\int_0^1\frac{\ln(1+y)\ln y}{1-y}-4\int_0^1\frac{\ln(1+y)\ln y}{1+y}+2\ln2\zeta(2)
\end{align}
where the first integral is
$$\int_0^1\frac{\ln y\ln(1+y)}{1-y}\ dy=\zeta(3)-\frac32\ln2\zeta(2)$$
and the second integral is
$$\int_0^1\frac{\ln y\ln(1+y)}{1+y}\ dy=-\frac12\int_0^1\frac{\ln^2(1+y)}{y}dy=-\frac18\zeta(3)$$
Combine the results of the two integrals we get
$$\boxed{\sum_{n=1}^\infty\frac{H_n}{n^24^n}{2n\choose n}=\frac92\zeta(3)-4\ln2\zeta(2)}$$
If we differentiate both sides of $\int_0^1 x^{n-1}\ln(1-x)dx=\frac{H_n}{n}$ we get
$$ \int_0^1x^{n-1}\ln x\ln(1-x)dx=\frac{H_n}{n^2}+\frac{H_n^{(2)}-\zeta(2)}{n}\tag2$$
Now multiply both sides of $(2)$ by $ \frac{1}{4^n}{2n\choose n}$ the sum up from $n=1$ to $\infty$ we get
$$\sum_{n=1}^\infty \frac{H_n}{n^24^n}{2n\choose n}+\sum_{n=1}^\infty \frac{H_n^{(2)}}{n4^n}{2n\choose n}-\zeta(2)\sum_{n=1}^\infty \frac{1}{n4^n}{2n\choose n}\\=\int_0^1\frac{\ln x\ln(1-x)}{x}\sum_{n=1}^\infty \frac{\binom{2n}n}{4^n}x^n\ dx=\int_0^1\frac{\ln x\ln(1-x)}{x}\left(\frac{1}{\sqrt{1-x}}-1\right)\ dx\\=\underbrace{\int_0^1\frac{\ln x\ln(1-x)}{x\sqrt{1-x}}dx}_{\text{Beta function:}7\zeta(3)-6\ln2\zeta(2)}-\underbrace{\int_0^1\frac{\ln x\ln(1-x)}{x}dx}_{\zeta(3)}$$
Substitute $\sum_{n=1}^\infty\frac{H_n}{n^24^n}{2n\choose n}=\frac92\zeta(3)-4\ln2\zeta(2)$ and $\sum_{n=1}^\infty\frac{1}{n4^n}{2n\choose n}=2\ln2$ we get
$$\boxed{\sum_{n=1}^\infty\frac{H_n^{(2)}}{n4^n}{2n\choose n}=\frac32\zeta(3)}$$