We derive a dramatic improvement over a comment that suspected even $k= 3\uparrow^{g_{63}-1}3$ is not enough iterations for $f^k(\text{googolplex}) > \text{Graham's number}$, where $f$ is the factorial function.
For convenience in writing Knuth's up-arrows, we use the operator notation $$[a]b = 3\uparrow^a b,$$
so Graham's number $(g_{64})$ is defined by the recursion $$g_0 = 4\\ g_{n+1} = [g_n]3.$$
We show that Graham's number can be written as an exactly specified
number of iterations of the
tetration operator $([2])$:
$$\text{Graham's number } = [2]^t 1 $$ and therefore that
$$\text{Graham's number } \gt f^{t-3}(\text{googolplex})$$ because $\
[2]^3 1 > \text{googolplex}\ $ and $\ [2]n > n!\ $ for all positive
integers $n$.
Before proceeding to calculate $t$, we state some properties of the hyperoperators $[p]$. Associating from the right, these satisfy the following recursion for $a,b\in Z_{>0}$:
$$[a]b =
\begin{cases}
3 & \text{if } b=1\\
3^b & \text{if }a=1\\
[a-1][a](b-1) & \text{otherwise}
\end{cases}\tag{E0}$$
which implies the identities
$$\begin{align}
[a]b &= [a-1]^b 1 &(a\ge 2,\ b \ge 1)\tag{E1}\\
[a]b &= [a-2]^{[a](b-1)}1 &(a\ge 3,\ b \ge 2)\tag{E2}
\end{align}$$
Aside: $(E1)$ is obtained by repeatedly applying $(E0)$ to itself, as
$$\begin{align}[a]b
&= [a-1][a](b-1)\\
&= [a-1][a-1][a](b-2)\\
&\cdots\\
&= [a-1]^{(b-1)}[a] 1\\
&= [a-1]^{(b-1)}[a-1] 1\\
&= [a-1]^b 1
\end{align}$$
and $(E2)$ is obtained by applying $(E1)$ to $(E0)$ as
$$[a]b = [\underbrace{a-1}_{A}]\underbrace{[a](b-1)}_{B} = [A]B = [A-1]^B 1 = [a-2]^{[a](b-1)}1.$$
General result:
If $p\ge 4\ $ and $\ q \le p-3\ $ are positive integers with opposite
parity, then $$[p]3 = [q]^t 1$$ where $$t=[q+2](b_j-1)\\
j={{p-q-1}\over{2}}$$ and $b_j$ is the last term in the very rapidly
increasing sequence $b_1 < b_2 < \dots < b_j$, given by the recursion
$$\begin{align} b_1 &= [p-1][p-1]1\\ b_i &=
[p-2i+1]^{[p-2i+3](b_{i-1}-1)-1}1\quad (1\lt i\le j).\\ \end{align}$$
Proof-sketch, using repeated application of the previous identity $E2$ until $[p]3$ is reduced to the form $[q]^t 1$:
$$\begin{align}
[p]3
&= [p-1]([p-1][p-1]1)\\
&= [a_1]b_1,\quad a_1 = p-1,\ b_1=[p-1][p-1]1\\
&= [a_1-2][a_1-2]^{[a_1](b_1-1)-1}1\\
&= [a_2]b_2,\quad a_2 = a_1 - 2=p-3,\ b_2 = [a_2]^{[a_1](b_1-1)-1}1\\
&= [a_2-2][a_2-2]^{[a_2](b_2-1)-1}1\\
&= [a_3]b_3,\quad a_3 = a_2 - 2=p-5,\ b_3 = [a_3]^{[a_2](b_2-1)-1}1\\
&...\\
&= [a_i-2]^{[a_i](b_i-1)},\quad a_i = a_{i-1} - 2=p-2i+1,\ b_i = [a_i]^{[a_{i-1}](b_{i-1}-1)-1}1\\
&...\\
&= [q]^{[q+2](b_j-1)}1,\quad q = a_j-2=p-2\cdot j-1\implies j={{p-q-1}\over{2}}\\
\end{align}$$
QED
Applying the above results to $p=g_{63}$ and $q=2$:
$$\text{Graham's number } = [2]^t 1 > f^{t-3}(\text{googolplex})$$
where $$t=[4](b_j-1)\\
j={{g_{63}-3}\over{2}}$$ and $b_j$ is the last term in the very long and rapidly
increasing sequence $b_1 < b_2 < \dots < b_j$ given by the recursion
$$\begin{align} b_1 &= [g_{63}-1][g_{63}-1]1\\ b_i &=
[g_{63}-2i+1]^{[g_{63}-2i+3](b_{i-1}-1)-1}1\quad (1\lt i\le j).\\ \end{align}$$
NB: We have $t = [4](b_j-1) \gg b_i$ for each $b_i$ in the sequence $b_1 < b_2 < \dots < b_j$, where the number of terms is $j={{g_{63}-3}\over{2}}$, and already the second term is
$$b_2 = [g_{63}-3]^{[g_{63}-1]([g_{63}-1]3-1)-1}1.$$
Making some extremely crude simplifications, we have for example
$$k \le {[4]^{[6]^{[8]{\cdot^{\cdot^{\cdot^{[g_{63}-3]^Q 1}\cdot}\cdot}\cdot}1}1}1} \ \implies\ f^k (\text{googolplex}) \le \text{Graham's number}$$
where the topmost term is $Q = [g_{63}-1]([g_{63}-1]3-1)-1$
and the height of the "iteration tower" is ${g_{63}-3}\over 2$.