You lost a negative sign, but overall your work holds together.
In any number of dimensions, say $n\geq 2$,
$$\vec{\nabla}\left(\frac{1}{r}\right) = \frac{-r\hat{r}}{r^{3}}$$
has zero divergence for $r\neq 0$:
$$\Delta\left(\frac{1}{r}\right)=0 \mbox{ for } r\neq 0.$$
Physically this means that no electric field is being generated away from the origin, for example.
The only question, then, is what is happening at $r=0$, where you envision a point charge being located at the origin that is generating an electric field. How strong is that source?
We consider this problem by letting our domain $\Omega$ be an $n$-dimensional sphere of radius $R$ and letting $R\to 0^{+}$. The term in our integral that will work, if any such term exists, gives the strength of our point source, which in your context is the value of $\Delta \left(\frac{1}{r}\right)$ at the origin.
This is the context into which your computations fit. Your computations are correct: in determining the Laplacian of $\frac{1}{r}$ at the origin you look at a volume integral and turn it into a surface integral over the boundary of a ball of radius $R>0$, where again your focus is on what is happening as $R\to 0^{+}$.
You determine this by looking at
$$\int_{\Omega}\Delta\left(\frac{1}{r}\right)dV = \int_{\partial \Omega}\vec{\nabla}\left(\frac{1}{r}\right)\cdot \hat{r}dA = \int_{\partial \Omega}\frac{-R\hat{r}}{R^{3}}\cdot \hat{r}dA = \int_{\partial \Omega}\frac{-1}{R^{2}}dA.$$
The spherical area element in $n$ dimensions has a factor of $R^{n-1}$ with additional angular terms that, big-picture, we don't care about. The important point is that when $n=3$ the radial factors cancel out perfectly and we are left with a point source that has an intrinsic strength that is easily defined as it can be measured as the flux of electric field through a sphere of any radius about the point charge, since there is no $R$ is our answer.
For $n\neq 3$ the easiest, most accurate, thing to say is simply that we don't have a particularly meaningful way of defining the strength of a point source as we can longer meaningfully connect it to the flux out through a sphere of arbitrary radius: the flux now depends upon $R$.
If you attempt to define the "intrinsic strength" of a point source as the flux through a sphere of radius $R$ as $R\to 0^{+}$, then we find that:
When $n=2$ there is an overall factor of $\frac{1}{R}$ that goes to $\infty$ as $R\to 0^{+}$, so the "intrinsic strength" of the point source is infinite.
When $n\geq 4$ there is an overall factor of $R^{n-3}$ that goes to $0$ as $R\to 0^{+}$, so the "intrinsic strength" of the point source is $0$.
These results make intuitive sense in that with fewer dimensions there is less "space" for the electric field to dissipate, so that $n=2$ is too cramped and the "intrinsic strength" is infinite, $n\geq 4$ is too spacious and the "intrinsic strength" is $0$, and $n=3$ is just right, which makes a proper definition of the strength of a point charge possible.
Thanks for the detailed answer
– Ragnar May 24 '15 at 17:37